by Hester, Gavin, DeLazzer, T. N., Yahne, D. R., Sarkis, C. L., Zhao, H. D., Rivera, J. A. Rodriguez, Calder, S. and Ross, K. A.
Abstract:
Ising-like spin-1/2 magnetic materials are of interest for their ready connection to theory, particularly in the context of quantum critical behavior. In this work we report detailed studies of the magnetic properties of a member of the rare earth pyrosilicate family, D-Er2Si2O7, which is known to display a highly anisotropic Ising-like g-tensor and effective spin-1/2 magnetic moments. We used powder neutron diffraction, powder inelastic neutron spectroscopy (INS), and single crystal AC susceptibility to characterize its magnetic properties. Neutron diffraction enabled us to determine the magnetic structure below the known transition temperature (T (N) = 1.9 K) in zero field, confirming that the magnetic state is a four-sublattice antiferromagnetic structure with two non-collinear Ising axes, as was previously hypothesized. Our powder INS data revealed a gapped excitation at zero field, consistent with anisotropic (possibly Ising) exchange. An applied field of 1 T produces a mode softening, which is consistent with a field-induced second order phase transition. To assess the relevance of D-Er2Si2O7 to the transverse field Ising model, we performed AC susceptibility measurements on a single crystal with the magnetic field oriented in the direction transverse to the Ising axes. This revealed a transition at 2.65 T at 0.1 K, a field significantly higher than the mode-softening field observed by powder INS, showing that the field-induced phase transitions are highly field-direction dependent as expected. These measurements suggest that D-Er2Si2O7 may be a candidate for further exploration related to the transverse field Ising model.
Reference:
Hester, Gavin, DeLazzer, T. N., Yahne, D. R., Sarkis, C. L., Zhao, H. D., Rivera, J. A. Rodriguez, Calder, S. and Ross, K. A., "Magnetic properties of the Ising-like rare earth pyrosilicate: D-Er2Si2O7", In JOURNAL OF PHYSICS-CONDENSED MATTER, vol. 33, no. 40, 2021.
Bibtex Entry:
@article{ WOS:000680173400001,
Author = {Hester, Gavin and DeLazzer, T. N. and Yahne, D. R. and Sarkis, C. L. and
Zhao, H. D. and Rivera, J. A. Rodriguez and Calder, S. and Ross, K. A.},
Title = {Magnetic properties of the Ising-like rare earth pyrosilicate:
D-Er2Si2O7},
Journal = {JOURNAL OF PHYSICS-CONDENSED MATTER},
Year = {2021},
Volume = {33},
Number = {40},
Month = {OCT 6},
Abstract = {Ising-like spin-1/2 magnetic materials are of interest for their ready
connection to theory, particularly in the context of quantum critical
behavior. In this work we report detailed studies of the magnetic
properties of a member of the rare earth pyrosilicate family,
D-Er2Si2O7, which is known to display a highly anisotropic Ising-like
g-tensor and effective spin-1/2 magnetic moments. We used powder neutron
diffraction, powder inelastic neutron spectroscopy (INS), and single
crystal AC susceptibility to characterize its magnetic properties.
Neutron diffraction enabled us to determine the magnetic structure below
the known transition temperature (T (N) = 1.9 K) in zero field,
confirming that the magnetic state is a four-sublattice
antiferromagnetic structure with two non-collinear Ising axes, as was
previously hypothesized. Our powder INS data revealed a gapped
excitation at zero field, consistent with anisotropic (possibly Ising)
exchange. An applied field of 1 T produces a mode softening, which is
consistent with a field-induced second order phase transition. To assess
the relevance of D-Er2Si2O7 to the transverse field Ising model, we
performed AC susceptibility measurements on a single crystal with the
magnetic field oriented in the direction transverse to the Ising axes.
This revealed a transition at 2.65 T at 0.1 K, a field significantly
higher than the mode-softening field observed by powder INS, showing
that the field-induced phase transitions are highly field-direction
dependent as expected. These measurements suggest that D-Er2Si2O7 may be
a candidate for further exploration related to the transverse field
Ising model.},
DOI = {10.1088/1361-648X/ac136a},
Article-Number = {405801},
ISSN = {0953-8984},
EISSN = {1361-648X},
ORCID-Numbers = {Hester, Gavin/0000-0003-1444-4510},
Unique-ID = {WOS:000680173400001},
}